The key ingredient is the following theorem of Ulam:
Theorem: Let $\mu$ be a finite measure defined on the entire power set $P(\omega_1)$ which vanishes on singletons. Then $\mu=0$.
In particular, we can apply this to your setup as follows.
Corollary: Let $\nu$ be a Borel probability measure on $\omega_1$ which vanishes on singletons, and suppose $U\subset\omega_1$ can be written as a disjoint union of bounded open sets. Then $\nu(U)=0$.
Proof of Corollary from Theorem: Suppose $U=\bigcup_{\alpha<\omega_1} U_\alpha$ where the $U_\alpha$ are disjoint, bounded, and open. Define a measure $\mu$ on $P(\omega_1)$ by $\mu(A)=\nu(\bigcup_{\alpha\in A} U_\alpha)$ (this is well-defined since such a union is always open and a measure since the $U_\alpha$ are disjoint). Then $\mu$ vanishes on singletons since each $U_\alpha$ is bounded. Thus by the Theorem, $\mu=0$, and in particular $\nu(U)=\mu(\omega_1)=0$.
Now to prove your Lemma, let $K\subset\omega_1$ be any closed unbounded set and let $U=\omega_1\setminus K$. Enumerating the elements of $K$ in order as $(c_\alpha)_{\alpha<\omega_1}$, then we can partition $U$ into the bounded open sets $[0,c_0)$ and $(c_\alpha,c_{\alpha+1})$ as $\alpha$ ranges over all of $\omega_1$. Thus by the Corollary, $\nu(U)=0$ and so $\nu(K)=1$.
Finally, here is a proof of the Theorem. Suppose $\mu$ is nonzero. For each $\alpha<\omega_1$, let $f_\alpha:\alpha\to\omega$ be an injection. For $\beta<\omega_1$ and $n<\omega$, let $A_{\beta,n}=\{\alpha:f_\alpha(\beta)=n\}$. Note that for fixed $\beta$, $\bigcup_n A_{\beta,n}=\omega_1\setminus(\beta+1)$ (since $f_\alpha(\beta)$ is defined as long as $\alpha>\beta$), which has full measure since $\mu$ vanishes on countable sets. Thus for each $\beta$ there is some $n$ such that $A_{\beta,n}$ has positive measure. Since there are uncountably many $\beta$'s and only countably many $n$'s, then must be some fixed $n$ such that $A_{\beta,n}$ has positive measure for uncountably many different $\beta$. But for fixed $n$, the sets $A_{\beta,n}$ are disjoint since the functions $f_\alpha$ are injective. Since a finite measure cannot have an uncountable family of disjoint sets of positive measure, this is a contradiction.