No two people's neurons are wired the same way, but if you want to multiply 2-digit numbers together in your head, you can try using the following idea.
Given
$\quad n \,= 10 n_1 + n_0 \quad \;\;\,\text{ with } n_1, n_0 \;\,\in \{1,2,3,4,5,6,7,8,9\}$
$\quad m = 10 m_1 + m_0 \quad \text{ with } m_1, m_0 \in \{1,2,3,4,5,6,7,8,9\}$
To multiply $n \times m$,
1). Multiply the left digits and store in your L-register,
$\tag 1 L = n_1 \times m_1$
Regard the register $L$ as having a length of $2$ (pad on the left with $0$ if necessary).
2). Multiply the right digits and store in your R-register,
$\tag 2 R = n_0 \times m_0$
Regard the register $R$ as having a length of $2$ (pad on the left with $0$ if necessary).
3.) Split the $R$ register string into your $R1$ and $F$ registers,
$\tag 3 R = R1 \, || \, F$
Release the $R$ register to 'clear' memory.
4.) Concatenate the $R_1$ digit to the right of the $L$ and store in your T-register,
$\tag 4 T = L \, || \, R_1$
Release the $R_1$/$L$ registers to clear memory.
5). Add the '-outers' and '-inners' into your T1-register,
$\tag 5 T1 = [n_1 \times m_0] + [n_0 \times m_1]$
The number $T1$ in $\text{base-}10$ has length of at most $3$.
6). Add the two registers $T$ and $T1$ together, storing the results in 3-digit register $G$.
7). Say or think the answer,
$\tag 6 G \, || \, F$
Example 1: $73 \times 42$
Combining steps, you are saying in your head $280$, and, if nobody is looking, using your fingers to store $6$.
You add $14$ (outers) to $12$ (inners), saving $26$.
You add $280 + 26$ giving $306$.
You say the answer, $3,066$.
Example 2: $18 \times 17$
Combining steps, you are saying in your head $015$, and, if nobody is looking, using your fingers to store $6$.
You add $7$ (outers) to $8$ (inners), saving $15$.
You add $015 + 15$ giving $30$.
You say the answer, $306$.
Example 3: $64 \times 43$
Combining steps, you are saying in your head $241$, and, if nobody is looking, using your fingers to store $2$.
You add $18$ (outers) to $16$ (inners), saving $34$.
You add $241 + 34$ giving $275$.
You say the answer, $2,752$.
Example 4: $97 \times 97$
Combining steps, you are saying in your head $814$, and, if nobody is looking, using your fingers to store $9$.
You add $63$ (outers) to $63$ (inners), saving $126$.
You add $814 + 126$ giving $940$.
You say the answer, $9,409$.
The starting point for this technique can be found here:
$\quad$ What is the fastest way to multiply two digit numbers?