It is a classic result of B.H.Neumann that there is a continuum (that is, $2^{\aleph_0}$) of pairwise non-isomorphic two-generated groups†. That is, there is a continuum of groups with presentations of the form $\langle a, b\mid \mathbf{r}\rangle$, where $\mathbf{r}$ is the set of relators (so the set $\mathbf{r}$ normally generates the kernel of $F(a, b) \twoheadrightarrow G\cong\langle a, b;\mathbf{r}\rangle$).
It is relatively easy to convince yourself that if the set $\mathbf{r}$ is finite then there are only countably many such presentations (and so countable many two-generated, finitely presentable groups). What is less obvious is that there are only countably many recursively enumerable sets $\mathbf{r}$. Hence, of the continuum of two-generated groups, most are not even recursively presentable never mind finitely presentable!
I should say that the idea of "recursively presentable groups" seems rather odd, but there is a rather spectacular result of Graham Higman which says that a finitely generated group is recursively presentable if and only if it can be embedded into a finitely presentable group.
(I should say that this all implies basically the same results for free groups of rank greater than two.)
†B.H.Neumann, Some remarks on infinite groups, J. London Math. Soc. 12 (1937) 120-127,)